Growth and scintillation properties of Tm3+ doped Bi4Si3O12 single crystals
XUEFENG XIAO1,2,3,4,*
,
HUAN ZHANG1,2,
HAICHENG WEI1,2,
JIAYUE XU4,*
,
YAOQING CHU4,
BOBO YANG4,
XUEFENG ZHANG5
Affiliation
- Key Laboratory of Physics and Photoelectric Information Functional Materials Sciences and Technology, North Minzu University, Yinchuan, 750021, China
- College of Electric and Information Engineering, North Minzu University, Yinchuan, 750021, China
- School of Materials Science and Engineering, Tongji University, Shanghai 201804, China
- School of Materials Science and Engineering, Shanghai Institute of Technology, Shanghai, 201804, China
- Ningxia Ju Jing Yuan Crystal Technology Company Limited, Shizuishan 753000, China
Abstract
Doping with Tm3+ of 0.5mol%, 1.0mol%, 2.0mol% in the Bi4Si3O12 (BSO) crystals were grown by the modified vertical Bridgman method, respectively. The Bi4Si3O12:Tm(BSO:Tm) polycrystalline powders are prepared of using two step sintering method, namely sintered 12h at 800℃, cool to room temperature, after grinded, then sintered 8~12h at 850℃, used for crystal growth. The transmittance of Bi4Si3O12:Tm(BSO:Tm) crystals is about 80% and the optical quality of the crystal is same as the pure BSO crystal. The scintillation properties of BSO:Tm crystals are tested and analyzed. Pulse height measurements under γ-ray irradiation show that doping with 0.5 mol% Tm2O3 can increase the relative light yield of BSO from 5.0% to 5.2% of the CsI(Tl) crystal, consequently improving the ability to distinguish between particles. These results indicate that BSO:Tm crystals could be a promising candidate in some applications, such as electromagnetic and dual-readout calorimeters in nuclear or high energy physics.
Keywords
Bi4Si3O12 crystal, Crystal growth, Tm3+ ions, Scintillation characteristics, Relative light yield.
Citation
XUEFENG XIAO, HUAN ZHANG, HAICHENG WEI, JIAYUE XU, YAOQING CHU, BOBO YANG, XUEFENG ZHANG, Growth and scintillation properties of Tm3+ doped Bi4Si3O12 single crystals, Optoelectronics and Advanced Materials - Rapid Communications, 14, 7-8, July-August 2020, pp.367-371 (2020).
Submitted at: Dec. 12, 2019
Accepted at: Aug. 18, 2020